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Instrument
Description:
1)
Instrument Function.
The
ER-2 CNC counts particles in the approximate diameter range from 0.006 m
to 2 m. The instrument
operates by exposing the articles to saturated Flourinert vapor at 28 C
and then cooling the sample in a condenser at 5 C.
The supersaturation of the vapor increases as it is cooled and the
vapor condenses on the particles causing them to grow to sizes which are
easily detected. The
resulting droplets are passed through a laser beam and the scattered light
is detected. Individual
particles are counted (Wilson et al., 1983) and are referred to as
condensation nuclei (CN). Two
CN Counters are provided in the instrument.
One counts the particles after sampling from the atmosphere and the
second counts particles that have survived heating to 192C.
Lab experiments show that pure sulfuric acid particles smaller than
0.05 mm
are volatilized in the heater. The
heated channel detects when small particles are volatile and permits
speculation about the composition. The
CNC II contains an impactor collector which permits the collection of
particles on electron microscope grids for later analysis.
The collector consists of a two stages.
In the first stage the pressure of the sample is reduced by a
factor of two without loosing particles by impaction on walls.
The second stage consists of a thin plate impactor which collect
efficiently even at small Reynolds numbers.
The system collects particles as small as 0.02 m at WB-57F cruise
altitudes. As many as 25
samples can be collected in a flight.
2) Utility of the Data.
In the vicinity of the
tropopause, the mixing ratios of CN show strong gradients with latitude
and altitude. Thus they can
be useful tracers in transport experiments (Wilson, et al. 1991).
The heated and unheated CNC concentrations have provided important
information concerning emissions from aircraft (Fahey et al., 1995) and
have provided important information concerning new particle formation near
the tropical tropopause (Brock et al., 1993).
Aerosol composition also shows strong gradients near the tropopause
(Sheridan et al., 1994) and will be very informative concerning rocket
emissions.
3) Instrument Characteristics.
Accuracy. The instrument
has been calibrated with monodisperse aerosol carrying a single charge.
The ER-2 CNC and the electrometer agree to within 15%.
Sampling errors may increase the uncertainty but a variety of
comparisons suggests that total uncertainties are near 15%.
Precision. The precision
equals 1/ÖN
where N is the number of particles counted.
In many instances near the tropopause it is better than 3% at a one
Hertz data rate. At cruise
altitude, the precision may reach 15%.
If better precision is desired, it is necessary only to accumulate
over longer time intervals.
Response Time: Data are
acquired at 4 Hz. However the
response time depends upon the precision required to detect the change in
question. Small changes may
require longer times to detect.
Weight: Approximately 68 lbs.
References:
Brock,
C. A., P. Hamill, J. C. Wilson, H. H. Jonsson, K. R. Chan,"Particle
formation in the upper tropical troposphere: a source of nuclei for the
stratospheric aerosol," Science,
270, 1650-1653, (1995).
Fahey,
D. W., E. R. Keim, K. A. Boering, C. A. Brock, J. C. Wilson, H. H. Jonsson,
S. Anthony, T. F. Hanisco, P.
O. Wennberg, R. C. Miake-Lye, R. J. Salawitch, N. Louisnard, E. L.
Woodbridge, R. S. Gao, S. G. Donnelly, R. C. Wamsley, L. A. Del Negro, S.
Solomon, B. C. Daube, S. C. Wofsy, C. R. Webster, R. D. May, K. K. Kelly,
M. Loewenstein, J. R. Podolske, K. R. Chan, Emission Measurements of the
Concorde Supersonic Aircraft in the Lower Stratosphere, Science,
270,70-74(1995).
Sheridan,
P. J., Brock, C. A., Wilson J. C., “Aerosol particles in the upper
troposphere and lower stratosphere: Elemental composition and morphology
of individual particles in northern midlatitudes”
Geophysical Research Letters, 21, 2587-2590, 1994.
Wilson
J.C., Blackshear E.D., Hyun J.H., "The Function and Response of an
Improved Stratospheric Condensation Nucleus Counter," Journal
of Geophysical Research:
Oceans and Atmospheres 88:6781-6785, 1983.
Wilson,
J. C., Lai,W. T., Smith, S. D. "Measurements of condensation nuclei
above the jet stream: evidence for cross jet transport by waves and new
particle formation at high altitudes", Journal
of Geophysical Research, 96:17,415-17,423, 1991
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